George certainly something like 747-800's would be able to carry more payload. But 747's are not created equal - you cannot claim it would take a number of 747-800's, and then say that there aer "thousands" of 747's around that could be used when those 747's that are "around" are not -800's.
747-200 payload/range
747-400 payload/range
747-8 payload range (on page 12 of the brochure)
As you can see from those, maximum payload can NOT be carried to maximum range, plus you still have to factor in the weight of the equipment required to store and distribute the material on board the aircraft - which I think is likely to be a considerable portion of the available payload. How much I don't know, but you will need tanks strong enough to hold it against reasonable forces, piping and pumps, probably extra power supplies to run the pumps. And all these will have to be corrosion resistant, which will probably mean stainless steel rather than lightweight materials.
alternatively you could try to keep it entirely dry (ie remove all water, not stop it from being liquid) which would prevent it from forming corrosive compounds. I have no idea what that would take.
you are proposing to use SO2 - sulphur dioxide - which is a gas. Liquid SO2 can be used -
some of its characteristics are noted here - but as noted the liquid phase requires pressure to form in equilibrium with the gas phase - which means all those tanks, etc would have to be pressure vessels on top of all the other requirements - or kept at at -10 deg C or cooler and atmospheric pressure, which means insulated containers and cooling systems.
given what I do know about refrigerated and pressurised storage of liquids and gasses (strictly as a user) it would not surprise me if 2/3rds or more of the available payload was taken up with storage and handling equipment - that is just a guess on my part of course, but whatever the portion required it still has to be taken into account.
Other considerations:
-The 1% or so change in optical depth from your 1Tg injection is not so small as to be unnoticeable - you will have to inject less than that. How much less I don't know - so you'll have to figure that out, and then determine whether such smaller amount will manage to have any effect at all.
-1Tg of sulphur is not "background" - it is a measureable % increase in total atospheric sulpur injection 20-60 Mt (20-60Tg) of SOx per year (see the IPCC's
Scenarios for greenhouse gasses here)
-you still have to secretly produce and distribute 1Tg (1 million tonnes) of sulphur each year somehow. That is 25,000 truckloads at 40 tons each - or about 70 trucks per day. Even spread around 4 facilities that is and average of about 18 trucks per day per facility....carrying dangerous goods. And of course the comments above about the weight of handling equipment applies to the transports as well - whether trucks or rail or anything else.